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- W2947393788 endingPage "11017" @default.
- W2947393788 startingPage "11013" @default.
- W2947393788 abstract "Abstract Catalytic asymmetric cycloadditions of ambident Pd‐containing dipolar species with nucleophilic dipolarophiles, namely, inverse‐electron‐demand cycloadditions, are challenging and underdeveloped. Possibly, the inherent linear selectivity of Pd‐catalyzed intermolecular allylations and the lack of efficient chiral ligands are responsible for this limitation. Herein, two cycloadditions of such intermediates with deconjugated butenolides and azlactones were accomplished by using a novel chiral hybrid P,S‐ligand and hydrogen bonding. By doing so, highly functionalized, optically active dihydroquinol‐2‐ones were produced with generally high reaction efficiencies and selectivities. Preliminary DFT calculations were performed to explain the high enantio‐ and diastereoselectivities." @default.
- W2947393788 created "2019-06-07" @default.
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- W2947393788 creator A5050027776 @default.
- W2947393788 creator A5056050312 @default.
- W2947393788 creator A5061000219 @default.
- W2947393788 date "2019-07-04" @default.
- W2947393788 modified "2023-10-03" @default.
- W2947393788 title "Inverse‐Electron‐Demand Palladium‐Catalyzed Asymmetric [4+2] Cycloadditions Enabled by Chiral P,S‐Ligand and Hydrogen Bonding" @default.
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- W2947393788 doi "https://doi.org/10.1002/anie.201905993" @default.
- W2947393788 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31144410" @default.
- W2947393788 hasPublicationYear "2019" @default.
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