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- W2947558130 abstract "Nitrogen-containing heterocycles are especially considered “privileged” structural scaffolds for the development of new drugs. However, traditional methods of organic synthesis are mainly based on thermal cycloaddition reaction; thus, the exploration of new strategies for the rapid assembly of N-heterocycles under mild conditions is highly desirable. Here, we developed a new method that visible light along with 1 mol % cercosporin, which is one of the perylenequinonoid pigments with excellent properties of photosensitization and can be easily produced by a new isolated endophytic fungus Cercospora sp. JNU001 strain with high yield through microbial fermentation, catalyzes the synthesis of 1,2,3-thiadiazoles and 1,4,5,6-tetrahydropyridazines by a photocatalytic process with good regioselectivity and broad functional-group compatibility under mild conditions. Thus, a bridge between microbial fermentation and organic photocatalysis for the construction of nitrogen-containing heterocycles was set up in a sustainable, environmentally friendly manner." @default.
- W2947558130 created "2019-06-07" @default.
- W2947558130 creator A5003751341 @default.
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- W2947558130 creator A5082388713 @default.
- W2947558130 creator A5082759825 @default.
- W2947558130 creator A5086664284 @default.
- W2947558130 date "2019-05-23" @default.
- W2947558130 modified "2023-10-18" @default.
- W2947558130 title "Perylenequinonoid-Catalyzed [4 + 1] and [4 + 2] Annulations of Azoalkenes: Photocatalytic Access to 1,2,3-Thiadiazole/1,4,5,6-Tetrahydropyridazine Derivatives" @default.
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- W2947558130 doi "https://doi.org/10.1021/acs.joc.9b00545" @default.
- W2947558130 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31117482" @default.
- W2947558130 hasPublicationYear "2019" @default.
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