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- W2947584604 abstract "The bimetallic Pt-Sn catalysts are known to be the most efficient ones for propane dehydrogenation reaction; however, the synthesis of bimetallic Pt-Sn nanocluster (below 1 nm) with an alloy structure still remains a formidable challenge. An approach for the controllable synthesis of Pt-Sn nanocluster based on Surface Organometallic Chemistry on oxide concept is developed here, which involves two basic steps: the sequential grafting of Pt(COD)Me2 and HSnPh3 at the surface of dehydroxylated θ-Al2O leading to the formation of well-defined bimetallic surface compound consisting of [(AlO)Pt(COD)Me] and [(AlO)SnPh3] fragments, and the hydrogenolysis of this surface compound under a mild condition giving rise to the ultra-small bimetallic Pt-Sn cluster around 0.75 nm. The achieved Pt-Sn/θ-Al2O3 catalysts exhibit high activity, selectivity and stability in propane dehydrogenation to propylene." @default.
- W2947584604 created "2019-06-07" @default.
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- W2947584604 date "2019-06-01" @default.
- W2947584604 modified "2023-10-06" @default.
- W2947584604 title "Bimetallic Pt-Sn nanocluster from the hydrogenolysis of a well-defined surface compound consisting of [( AlO )Pt(COD)Me] and [( AlO )SnPh3] fragments for propane dehydrogenation" @default.
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- W2947584604 doi "https://doi.org/10.1016/j.jcat.2019.04.035" @default.
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