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• W2947601282 endingPage "117771" @default.
• W2947601282 startingPage "117771" @default.
• W2947601282 abstract "Abstract A unique urchin-like CoZnAl-LDH/RGO/g-C3N4 (LDH/RGO/CN) Z-scheme photocatalyst, which is fabricated by the hydrothermal synthesis of CoZnAl-LDH and the in situ loading of RGO and g-C3N4, is developed for the photocatalytic conversion of CO2. The special spiny external surface and hollow inner cavity endow LDH/RGO/CN with a significantly enhanced light-harvesting capacity. The well-distributed g-C3N4 nanosheets on the CoZnAl-LDH nanoplates, combined with RGO as an electron mediator, constructs an excellent heterosystem with numerous interfaces, efficient charge separation and highly exposed catalytic active sites. The Z-scheme charge-transfer process promotes the oxidizability and reducibility of CoZnAl-LDH and g-C3N4. Furthermore, the synergistic effect among the components contributes to intense adsorption and chemical activation towards CO2, which reduces the reaction barrier for CO2 photoreduction. As a result, the optimized LDH/RGO/CN exhibits highly efficient and selective photocatalytic CO2 conversion to CO. The special 3D urchin-like architecture paves a new way for design of photocatalyst with ideal performance." @default.
• W2947601282 created "2019-06-07" @default.
• W2947601282 creator A5008323996 @default.
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• W2947601282 creator A5088123991 @default.
• W2947601282 date "2019-10-01" @default.
• W2947601282 modified "2023-10-14" @default.
• W2947601282 title "Urchin-like hierarchical CoZnAl-LDH/RGO/g-C3N4 hybrid as a Z-scheme photocatalyst for efficient and selective CO2 reduction" @default.
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• W2947601282 doi "https://doi.org/10.1016/j.apcatb.2019.117771" @default.
• W2947601282 hasPublicationYear "2019" @default.
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