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• W2947852562 endingPage "1934578X1984997" @default.
• W2947852562 startingPage "1934578X1984997" @default.
• W2947852562 abstract "The water soluble organic carbon of the prevalent atmospheric aerosol sources (traffic exhausts, paved road dust, agricultural soil, native soil, wood combustion, epicuticular waxes from pine and broad-leaved trees, and pollen) has been characterized using 1 H (1-dimensional), 1 H- 1 H-correlation spectroscopy and 1 H- 13 C-heteronuclear single quantum correlation 2-dimensional (2D) nuclear magnetic resonance (NMR) spectroscopy. Traffic exhaust particles were mainly constituted of primary alcohols, carbohydrates, functionalized olefins, C3 and C4 oxy- and hydroxyl-carboxylic acids, and short-chain alkanes. Road dust was a mixture of soil particles and traffic components. Agricultural, natural, road dust, and traffic particles contained broad signals that were attributed to poly-carboxylic compounds typically found in humic compounds and humic-like substances. Traces of traffic particles (ie, peaks in the 7.3-7.5 ppm [phthalic acid derivatives] and signals found in the 0.5-3 ppm originating from functionalized carboxylic acids) were also found in natural soil dust. Long-chain (>C3) fatty acids and amino acids were found in road dust, natural soil, pine trees waxes, pollen, and woodburning. The aromatic region mainly constituted of lignin derivatives and cellulose/hemicellulose pyrolysis products (signals in 2D-NMR) in woodburning. Primary biogenic and woodburning particles were uniquely clustered as compared to traffic exhausts, road, agricultural, and natural dust based on the relative ratio of hydro-oxygenated functional groups (H-C-O and H-C-C=O) to the sum of aliphatics. Overall, source-specific NMR spectrometric fingerprints, functional composition profiles, and several organic compounds were identified allowing for the reconciliation of ambient organic aerosol sources including the degree of atmospheric aging." @default.
• W2947852562 created "2019-06-07" @default.
• W2947852562 creator A5004118829 @default.
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• W2947852562 date "2019-05-01" @default.
• W2947852562 modified "2023-09-25" @default.
• W2947852562 title "Nuclear Magnetic Resonance Characterization of Water Soluble Organic Carbon of Atmospheric Aerosol Types" @default.
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• W2947852562 doi "https://doi.org/10.1177/1934578x19849972" @default.
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