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• W2948283806 abstract "Abstract Polyanilines (pANIs), loaded with phosphotungstic acid (PTA), are pyrolyzed to get WO 3 or W 2 N (≈6 and ≈7 nm, respectively), which is well‐dispersed on pANI‐derived porous carbons (pDCs). Depending on the pyrolysis temperature, WO 3 /pDC, W 2 N/pDC, or W 2 N‐W/pDCs could be obtained selectively. pANI acts as both the precursor of pDC and the nitrogen source for the nitridation of WO 3 into W 2 N during the pyrolysis. Importantly, W 2 N could be obtained from the pyrolysis without ammonia feeding. The obtained W 2 N/pDC is applied as a heterogeneous catalyst for the oxidative desulfurization (ODS) of liquid fuel for the first time, and the results are compared with WO 3 /pDC and WO 3 /ZrO 2 . The W 2 N/pDC is very efficient in ODS with remarkable performance compared with WO 3 /pDC or WO 3 /ZrO 2 , which is applied as a representative ODS catalyst. For example, W 2 N/pDC shows around 3.4 and 2.7 times of kinetic constant and turnover frequency (based on 5 min of reaction), respectively, compared to that of WO 3 /ZrO 2 . Moreover, the catalysts could be regenerated in a facile way. Therefore, W 2 N/pDC could be produced facilely from pyrolysis (without ammonia feeding) of PTA/pANI, and W 2 N, well‐dispersed on pDC, can be suggested as a very efficient oxidation catalyst for the desulfurization of liquid fuel." @default.
• W2948283806 created "2019-06-14" @default.
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• W2948283806 date "2019-06-05" @default.
• W2948283806 modified "2023-10-01" @default.
• W2948283806 title "Tungsten Nitride, Well‐Dispersed on Porous Carbon: Remarkable Catalyst, Produced without Addition of Ammonia, for the Oxidative Desulfurization of Liquid Fuel" @default.
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• W2948283806 doi "https://doi.org/10.1002/smll.201901564" @default.
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