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• W2949167448 abstract "An enantioselective synthesis of tetraponerines T4, T6, T7, and T8 in 24−36% overall yield is described. Key steps in this synthesis are a Pd-catalyzed domino allylation and a Ru-catalyzed ring rearrangement. The effect of different substituents on the equilibrium of the metathesis rearrangement has been investigated. To complete the synthesis a sequence of Wacker oxidation and Takai olefination was used. The preparation of four representative tetraponerines differing in stereochemistry, ring size, and side chain employing five metal-organic reactions clearly demonstrates the efficiency of transition metals in organic synthesis." @default.
• W2949167448 created "2019-06-27" @default.
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• W2949167448 date "2000-09-26" @default.
• W2949167448 modified "2023-10-16" @default.
• W2949167448 title "Enantioselective Synthesis of Tetraponerines by Pd- and Ru-Catalyzed Domino Reactions" @default.
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• W2949167448 doi "https://doi.org/10.1021/ja001688i" @default.
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