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- W2949228052 abstract "New halohydrazidation and hydrazidopalladation reactions were developed that use the synthon N-acyl-N-tosylhydrazine. The intramolecular bromohydrazidation reactions of β,γ-unsaturated N-acyl-N-tosylhydrazines readily afforded pyrazolidinone ring systems that contained a tetrasubstituted carbon center, and the primary amine of the N-acyl-N-tosylhydrazine was shown to be a soft nucleophile. The similar bromohydrazidation reaction of γ,δ-unsaturated N-acyl-N-tosylhydrazine resulted in O-cyclization to give a lactone ring instead of N-cyclization to give a hydropyridazine ring system; however, the intramolecular hydrazidopalladation reaction predominantly afforded a hydropyridazine ring. The established catalytic hydrazidopalladation reaction was applicable to several multisubstituted alkenes to construct a tetrasubstituted carbon center possessing a nitrogen group." @default.
- W2949228052 created "2019-06-27" @default.
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- W2949228052 date "2015-02-16" @default.
- W2949228052 modified "2023-09-27" @default.
- W2949228052 title "ChemInform Abstract: N-Acyl-N-tosylhydrazine as a Synthon to Construct Tetrasubstituted Carbon Centers Possessing a Nitrogen Group." @default.
- W2949228052 cites W1905162160 @default.
- W2949228052 doi "https://doi.org/10.1002/chin.201509158" @default.
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