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- W2949441782 abstract "A similar viscosity dependence of the CIEEL efficiencies for the para- and meta-substituted spiroadamantyl dioxetanes 1 has been observed, which implies that an electron-transfer mechanism operates through solvent-caged species for both regioisomers. The pronounced difference in the chemiexcitation yields for the meta- and para-substituted dioxetanes is rationalized in terms of the much larger (ca. 200-fold) rate constant for the electron back-transfer (BET) step to afford the excited meta CIEEL emitter. An in-depth kinetic analysis of the viscosity effect on the excited-state generation for the para versus meta regioisomers supports this conclusion." @default.
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- W2949441782 date "2000-09-14" @default.
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- W2949441782 title "The Effect of <i>meta</i> versus <i>para</i> Substitution on the Efficiency of Chemiexcitation in the Chemically Triggered Electron-Transfer-Initiated Decomposition of Spiroadamantyl Dioxetanes" @default.
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- W2949441782 doi "https://doi.org/10.1021/jo000495a" @default.
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