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- W2949454976 abstract "Abstract The polarized absorption spectrum of single crystals of NiTa2O6 has been measured from 6000 to 28 000 cm−1 at various temperatures from 300 to 10 K. All the observed absorption regions are due to electronic transitions mainly localized on the Ni2+ ions. The first band system in the region 6000–10500 cm−1 corresponds to a transition which occurs mainly by magnetic dipole mechanism. The band systems in the other regions are due to vibronic transitions. By applying our method of analysis of the site geometry based on symmetry descent, we deduce that the Oh→D2h distortion of NiO6n− can be decomposed into two contributions related to the steps Oh→D4h and D4h→D2h and that the second contribution is much larger than the first. Successively we give an explanation for most of the features of the spectra by considering only the D4h→D2h perturbation and the vibronic interactions. The effect of the spin-orbit coupling has also been considered." @default.
- W2949454976 created "2019-06-27" @default.
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- W2949454976 date "2010-08-20" @default.
- W2949454976 modified "2023-09-26" @default.
- W2949454976 title "ChemInform Abstract: The Electronic Spectrum of NiTa2O6" @default.
- W2949454976 cites W1995056517 @default.
- W2949454976 doi "https://doi.org/10.1002/chin.199319014" @default.
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