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• W2949678259 startingPage "1906" @default.
• W2949678259 abstract "In spite of the importance of ligand/copper-catalyzed arylations of nucleophiles in organic chemistry, the structural and electronic features that make a ligand efficient in these reactions have not been determined until now. In this work, several bidentate ligands involving pyridine and/or imine nitrogen binding sites such as our lead ligand 1 have been synthesized, and tested in phenol arylations with a view to highlight relationships between the structure of the chelates and their efficacy. This study allowed us to more precisely define the role of each type of N-binding site during the catalytic process, and to discover new efficient ligands. Among them, the iminopyridine 6a, which is cheap and easy-to-prepare in high yield, is very attractive for industrial applications. Some examples of its field of application are presented here. In the future, the development of this work could allow a more rational design of efficient ligands in arylation reactions, without resorting to classical ligand screening." @default.
• W2949678259 created "2019-06-27" @default.
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• W2949678259 date "2007-08-06" @default.
• W2949678259 modified "2023-10-18" @default.
• W2949678259 title "Nitrogen Ligands in Copper-Catalyzed Arylation of Phenols: Structure/Activity Relationships and Applications" @default.
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• W2949678259 doi "https://doi.org/10.1002/adsc.200600628" @default.
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