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- W2949742495 abstract "To develop high-performance lithium-sulfur (Li−S) batteries, designing and exploring an advanced sulfur cathode with a conductive and polar robust framework is highly significant to suppress the “shuttle effect” of polysulfides and enhance the utilization of active sulfur. Herein, a multifunctional conductive nanohybrid, which acts as a sulfur host, is rationally constructed by inserting/intertwining carbon nanotubes (CNTs) onto Co-embedded N-doped porous dual carbon polyhedrons derived from a resorcinol-formaldehyde (RF) polymer layer enwrapping ZIF-67 metal-organic frameworks (MOFs) (Co, N−C@RFC/CNTs). The porous carbon polyhedrons can accommodate a high amount of sulfur owing to their large inner void space; the RF coating carbon layer and the CNTs effectively increase the conductivity and build a network for providing smooth ions/e− pathways; In addition, the polar Co particles and electronegative N heteroatoms synergistically strengthen the chemical adsorption of polysulfides and accelerate the redox reaction of the sulfur cathode. Benefiting from these advantages, the as-fabricated Co, N−C@RFC/CNTs/S cathode delivers a high reversible capacity of 1373.7 mAh g−1 at 0.1 C, an impressive rate performance with 659.2 mAh g−1 at 2.0 C, and an outstanding cycling stability with an ultralow capacity decay rate of 0.041 % per cycle for 500 cycles at 1.0 C. This work provides a facile and high-efficiency approach to fabricating excellent-performance storage materials based on an MOF precursor." @default.
- W2949742495 created "2019-06-27" @default.
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- W2949742495 date "2019-07-01" @default.
- W2949742495 modified "2023-09-25" @default.
- W2949742495 title "A Porous Carbon Polyhedron/Carbon Nanotube Based Hybrid Material as Multifunctional Sulfur Host for High‐Performance Lithium‐Sulfur Batteries" @default.
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- W2949742495 doi "https://doi.org/10.1002/celc.201900744" @default.
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