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• W2949847768 endingPage "2430" @default.
• W2949847768 startingPage "2420" @default.
• W2949847768 abstract "The composition and synthesis conditions of the (Li/Na)CoO2 phase with an ordered 1:1 Li/Na stacking alternating with CoO2 slabs were determined from a careful study of the P2-Na∼0.7CoO2−O3-LiCoO2 system. An in situ X-ray diffraction (XRD) thermal study emphasizes the metastable character of this phase that can be stabilized only by very fast quenching. Its composition, (Li0.42Na0.37)CoO2, is significantly different from the ideally expected one, (Li0.50Na0.35)CoO2, and its structure, confirmed by Rietveld refinement of the XRD pattern, presents an ideal alternate ordering of lithium, cobalt, and sodium layers within OP4-type oxygen packing. The presence of vacancies in both alkali-ion layers was confirmed by electrochemical intercalation of lithium and sodium. For the first time, a new type of layered oxide exhibiting OPP9-type oxygen packing was evidenced. Between the CoO2 slabs, alkali ions are intercalated in the following order: Liocta−Naprism−Naprism. This material crystallizes in the R3̅m space group with ahex = 2.828 Å and chex = 46.85 Å cell parameters." @default.
• W2949847768 created "2019-06-27" @default.
• W2949847768 creator A5014397795 @default.
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• W2949847768 date "2011-02-18" @default.
• W2949847768 modified "2023-10-15" @default.
• W2949847768 title "Reinvestigation of the OP4-(Li/Na)CoO₂-Layered System and First Evidence of the (Li/Na/Na)CoO₂ Phase with OPP9 Oxygen Stacking" @default.
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• W2949847768 doi "https://doi.org/10.1021/ic102218w" @default.
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• W2949847768 hasPublicationYear "2011" @default.
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