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• W2949894744 startingPage "214105" @default.
• W2949894744 abstract "We outline a novel numerical method, called Ultrafast Ultrafast (UF$^2$), for calculating the $n^text{th}$-order wavepackets required for calculating n-wave mixing signals. The method is simple to implement, and we demonstrate that it is computationally more efficient than other methods in a wide range of use cases. Resulting spectra are identical to those calculated using the standard response function formalism but with increased efficiency. The computational speed-ups of UF$^2$ come from (a) non-perturbative and costless propagation of the system time-evolution (b) numerical propagation only at times when perturbative optical pulses are non-zero and (c) use of the fast Fourier transform convolution algorithm for efficient numerical propagation. The simplicity of this formalism allows us to write a simple software package that is as easy to use and understand as the Feynman diagrams that organize the understanding of $n$-wave mixing processes." @default.
• W2949894744 created "2019-06-27" @default.
• W2949894744 creator A5004512332 @default.
• W2949894744 creator A5032568868 @default.
• W2949894744 date "2019-06-07" @default.
• W2949894744 modified "2023-09-24" @default.
• W2949894744 title "Numerical method for nonlinear optical spectroscopies: Ultrafast ultrafast spectroscopy" @default.
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• W2949894744 doi "https://doi.org/10.1063/1.5094062" @default.
• W2949894744 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31176339" @default.
• W2949894744 hasPublicationYear "2019" @default.
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