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• W2949982010 abstract "Aromatic secondary amides such as benzanilide (1) exist in a trans-amide form both in the crystal and in the solution, whereas N-methylbenzanilide (2) exists in cis form in the crystal, and predominantly in a cis form in the solution. Similar cis conformational preferences were observed in aromatic N,N'-dimethylated ureas and guanidines, in which two aromatic rings are located face to face. The cis preferences of N-methylated amides, ureas and guanidines could be utilized to construct interesting aromatic architecture. N,N',N''-Trimethyl-N,N',N''-triphenyl-1,3,5-benzenetricarboxamide (20) and a cyclic triamide (24) have crystal structures in which three N-phenyl groups direct to the same orientation (syn conformation). 1,2-Bis(N-benzoyl-N-methylamino)benzene (22), which have no fixed asymmetric center, afforded chiral crystals by simple recrystallization. Furthermore, aromatic multi-layered structures could be built and applied to obtain aromatic molecules which have potent DNA-binding ability." @default.
• W2949982010 created "2019-06-27" @default.
• W2949982010 creator A5073163009 @default.
• W2949982010 date "2001-02-01" @default.
• W2949982010 modified "2023-09-25" @default.
• W2949982010 title "Discovery of cis-Preference of Aromatic N-Methylamides and Its Application to Molecular Constructions" @default.
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• W2949982010 doi "https://doi.org/10.1248/yakushi.121.117" @default.
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