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• W2950017880 abstract "The enantioselective synthesis of cladospolide B, C, and (ent)-cladospolide D has been achieved in 11−15 steps from 1-nonyne. The route relies upon an alkyne zipper reaction to relay an ynone and dienoate functional groups across a nine carbon fragment, which enables a highly enantioselective Noyori ynone reduction and a diastereo- and regioselective Sharpless dihydroxylation of a dienoate. In addition to being a flexible approach to three members of the cladospolide natural products, this route for the first time correctly established the structure for cladospolide D." @default.
• W2950017880 created "2019-06-27" @default.
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• W2950017880 date "2009-02-04" @default.
• W2950017880 modified "2023-10-07" @default.
• W2950017880 title "De Novo Asymmetric Synthesis of Cladospolide B−D: Structural Reassignment of Cladospolide D via the Synthesis of its Enantiomer" @default.
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• W2950017880 doi "https://doi.org/10.1021/ol9000119" @default.
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