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• W2950108800 abstract "<div>A combination of the temporally- and spatially-resolved phonon spectroscopy has enabled calibration of hydrogen bond transition from the vibration mode of heavy water to the core-shelled nanodroplet and the sub-nanosized ionic hydration shell in terms of phonon abundance-lifetime-stiffness. It is uncovered that charge injection by salt solvation and skin formation by molecular undercoordination (often called confinement) share the same supersolidity of H–O (D–O as a probe) bond contraction, O:H elongation, and electron polarization. The bond transition stems the solution viscosity, surface stress, and slows down the molecular dynamics. The skin reflection further hinders phonon energy dissipation and thus lengthens the phonon lifetime of the nanodroplet.</div>" @default.
• W2950108800 created "2019-06-27" @default.
• W2950108800 creator A5087389582 @default.
• W2950108800 date "2018-10-25" @default.
• W2950108800 modified "2023-09-27" @default.
• W2950108800 title "Phonon Abundance-Stiffness-Lifetime Transition from the Mode of Heavy Water to Its Confinement and Hydration" @default.
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• W2950108800 doi "https://doi.org/10.26434/chemrxiv.7246946" @default.
• W2950108800 hasPublicationYear "2018" @default.
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