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- W2950119157 abstract "ConspectusIndole alkaloids, one of the largest classes of alkaloids, serve as an important and rich source of pharmaceuticals and have inspired synthetic chemists to develop novel chemical transformations and synthetic strategies. Many biologically active natural products contain challenging indoline scaffolds, which feature a C3 all-carbon quaternary stereocenter that is often surrounded by a complicated polycyclic ring system. The creation of this quaternary stereocenter creates an inherent synthetic challenge because the substituents on the carbon center cause high steric repulsion. In addition, the presence of nitrogen atoms within the surrounding polycyclic rings can lead to synthetic difficulties.Oxidative coupling between two sp3-hybridized carbon anions provides a unique and powerful method for building C–C single bonds, especially for generating a C–C bond that joins one or two vicinal quaternary stereocenters. Although chemists have known of this transformation for a long time, they have only ap..." @default.
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- W2950119157 date "2015-05-01" @default.
- W2950119157 modified "2023-09-23" @default.
- W2950119157 title "ChemInform Abstract: Intramolecular Dearomative Oxidative Coupling of Indoles: A Unified Strategy for the Total Synthesis of Indoline Alkaloids" @default.
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- W2950119157 doi "https://doi.org/10.1002/chin.201521295" @default.
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