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- W2950129105 abstract "Heating a range of suitably substituted diazoacetoacetates produced a family of 2-(1,3-dioxolan-2-yl)phenyl ketenes that, under thermal conditions, smoothly underwent a [1,5]-H shift/6π-electrocyclic ring-closure sequence to give 1H-2-benzopyrans. The application of such processes to ketenes, produced by replacing the phenyl scaffolding with a thiophene ring, afforded thienopyrans. The aza-Wittig reaction of these 2-(1,3-dioxolan-2-yl)phenyl and thienyl ketenes with N-aryliminophosphoranes provided analogous ketenimines that transform into the respective 1(2H)isoquinolinones and thienopyridinones under similar thermal conditions, following the same type of cascade sequence." @default.
- W2950129105 created "2019-06-27" @default.
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- W2950129105 date "2013-12-02" @default.
- W2950129105 modified "2023-10-18" @default.
- W2950129105 title "Tandem Processes in<i>C</i>-Aryl Ketenes and Ketenimines Triggered by [1,5]-Hydride-Like Migration of an Acetalic Hydrogen Atom" @default.
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- W2950129105 doi "https://doi.org/10.1002/ejoc.201301501" @default.
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