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• W2950168640 abstract "The phototransformations of a few 2,3-diaroylaziridines and 2-aryl-3-aroylaziridines have been studied by steady-state photolysis and product analysis. The formation of various photoproducts could be substantiated by ring opening via C−C bond cleavage (leading to azomethine ylides), intramolecular hydrogen abstraction, and C−N bond cleavage. Isolation of stereospecific 3-pyrroline derivatives from the photoreaction of benzoylaziridines in the presence of DMAD confirms our previous results concerning the azomethine ylides as major transient intermediates, produced under laser pulse photoexcitation. Dimethyl 1-cyclohexyl-2-benzoylpyrrole-3,4-dicarboxylate (25), one of the photoadducts derived from the reaction of 1a and 1b with DMAD undergoes a novel and unusual photorearrangement to give dimethyl 2-(1-benzoylcyclohexyl)pyrrole-3,4-dicarboxylate (27), the structure of which was confirmed through X-ray crystallographic analysis." @default.
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• W2950168640 date "1996-01-01" @default.
• W2950168640 modified "2023-10-16" @default.
• W2950168640 title "Phototransformations of <i>C</i>-Benzoylaziridines. Dipolarophilic Trapping of Photogenerated Azomethine Ylides¹" @default.
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• W2950168640 doi "https://doi.org/10.1021/jo952047m" @default.
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