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Matches in SemOpenAlex for { <https://semopenalex.org/work/W2950219639> ?p ?o ?g. }

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• W2950219639 abstract "A general and efficient rhodium-catalyzed asymmetric cyanide-free hydrocyanation of alkenes has been developed. Based on the asymmetric hydroformylation/condensation/aza-Cope elimination sequences, a broad scope of substrates including mono-substituted, 1,2-, and 1,1-disubstituted alkenes (involving natural product R- and S-limonene) were employed, and a series of valuable chiral nitriles are prepared with high yields (up to 95 %) and enantioselectivities (up to 98 % ee). Notably, the critical factor to achieve high enantioseletivies is the addition of catalytic amount of benzoic acid. This novel methodology provides an efficient and concise synthetic route to the intermediate of vildagliptin and anagliptin." @default.
• W2950219639 created "2019-06-27" @default.
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• W2950219639 date "2019-07-09" @default.
• W2950219639 modified "2023-10-09" @default.
• W2950219639 title "Asymmetric Hydrocyanation of Alkenes without HCN" @default.
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• W2950219639 doi "https://doi.org/10.1002/anie.201906111" @default.
• W2950219639 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31209994" @default.
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