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- W2950261657 abstract "Gambierol, a representative of the marine ladder toxin family, consists of eight ether rings, 18 stereocenters, and two challenging pyranyl rings having methyl groups that are in a 1,3-diaxial orientation to one another. Herein we describe the generation of gambierol's A-C and F-H ring systems and demonstrate the versatility of the glycosyl anhydride, enol ether-olefin RCM strategy to fused polycyclic ethers. This work has both enabled us to generate sufficient quantities of the gambierol precursors and has enabled us to better understand the chemical transformations that were key to these efforts. Fundamental work included efforts to C-glycosides and C-ketosides, Claisen rearrangements, and enol ether-olefin RCM reactions." @default.
- W2950261657 created "2019-06-27" @default.
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- W2950261657 date "2006-05-23" @default.
- W2950261657 modified "2023-10-17" @default.
- W2950261657 title "Total Synthesis of Gambierol: The Generation of the A—C and F—H Subunits by Using a C-Glycoside Centered Strategy." @default.
- W2950261657 cites W2035118130 @default.
- W2950261657 doi "https://doi.org/10.1002/chin.200621214" @default.
- W2950261657 hasPublicationYear "2006" @default.
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