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- W2950302893 abstract "Bare FeO+ reacts in the gas phase with benzene at collision rate (k = 1.3 × 10−9 cm3 molecule−1 s−1), giving rise to the formation of Fe(C6H4)+/H2O(5%), Fe(C5H6)+/CO(37%), Fe(C5H5)+/CO/H. (2%), and Fe+/C6H5OH (56%). Neither the reaction rate nor the product distribution are subject to a significant kinetic isotope effect, thus, ruling out several mechanistic variants described in the literature to the operative for ‘analogous’ arene oxidation processes in solution. A mechanism is suggested which is in keeping with the experimental findings, and which also accounts for some remarkable results obtained, when two [Fe, C6,H6H6O]+ isomers are generated and subjected to a neutralization-re-ionization experiment in the gas phase." @default.
- W2950302893 created "2019-06-27" @default.
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- W2950302893 date "1992-06-24" @default.
- W2950302893 modified "2023-10-16" @default.
- W2950302893 title "Benzene Oxidation by ‘Bare’ FeO<sup>+</sup>in the Gas Phase" @default.
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- W2950302893 doi "https://doi.org/10.1002/hlca.19920750429" @default.
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