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- W2950387615 abstract "Two kinds of oxygen-deficient phases around LaNiO2.5 were obtained by a low-temperature H2 reduction of perovskite-type LaNiO3. An antiferromagnetic LaNiO2.5 with TN 140 K seems to be stoichiometric and a small amount of excess oxygen leads to a new ferromagnetic phases. A structural refinement has revealed that the former (space group C 2/c) comprised one-dimensionally linked NiO6 octahedra along the c-axis and NiO4 square-planars connecting the octahedra chains. A cooperative Jahn–Teller distortion was observed in both coordination polyhedra, which suggested that LaNiO2.5 has octahedral Ni3+ ions with the low-spin state and square-planar Ni+ ions. Its magnetic property and XPS spectrum support this model. The new ferromagnetism with Tc 230 K could be understood due to a slight canting in the antiferromagnetic interaction between the octahedra and the square-planes." @default.
- W2950387615 created "2019-06-27" @default.
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- W2950387615 date "2010-08-19" @default.
- W2950387615 modified "2023-09-26" @default.
- W2950387615 title "ChemInform Abstract: Synthesis, Crystal Structure, and Properties of Oxygen-Deficient Lanthanum Nickelate LaNiO3-x (0 ≤ x ≤ 0.5)." @default.
- W2950387615 cites W1981795447 @default.
- W2950387615 doi "https://doi.org/10.1002/chin.199428030" @default.
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