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• W2950403265 startingPage "568" @default.
• W2950403265 abstract "Describing the kinetics of polymer reactions, such as the formation of loops and hairpins in nucleic acids or polypeptides, is complicated by the structural dynamics of their chains. Although both intramolecular reactions, such as cyclization, and intermolecular reactions have been studied extensively, both experimentally and theoretically, there is to date no exact explicit analytical treatment of transport-limited polymer reaction kinetics, even in the case of the simplest (Rouse) model of monomers connected by linear springs. We introduce a new analytical approach to calculate the mean reaction time of polymer reactions that encompasses the non-Markovian dynamics of monomer motion. This requires that the conformational statistics of the polymer at the very instant of reaction be determined, which provides, as a by-product, new information on the reaction path. We show that the typical reactive conformation of the polymer is more extended than the equilibrium conformation, which leads to reaction times significantly shorter than predicted by the existing classical Markovian theory." @default.
• W2950403265 created "2019-06-27" @default.
• W2950403265 creator A5007118333 @default.
• W2950403265 creator A5038635374 @default.
• W2950403265 creator A5080309785 @default.
• W2950403265 date "2012-06-10" @default.
• W2950403265 modified "2023-09-25" @default.
• W2950403265 title "Non-Markovian polymer reaction kinetics" @default.
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• W2950403265 doi "https://doi.org/10.1038/nchem.1378" @default.
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• W2950403265 hasPublicationYear "2012" @default.
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