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• W2950441723 abstract "One challenge in developing the next generation of lithium-ion batteries is the replacement of organic electrolytes, which are flammable and most often contain toxic and thermally unstable lithium salts, with safer, environmentally friendly alternatives. Recently developed Water-in-Salt Electrolytes (WiSEs) were found to be a promising alternative, having also enhanced electrochemical stability. In this work, we develop a simple modified Poisson-Fermi theory, which demonstrates the fine interplay between electrosorption, solvation, and ion correlations. The phenomenological parameters are extracted from molecular simulations, also performed here. The theory reproduces the electrical double layer structure of WiSEs with remarkable accuracy." @default.
• W2950441723 created "2019-06-27" @default.
• W2950441723 creator A5027359414 @default.
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• W2950441723 date "2018-08-18" @default.
• W2950441723 modified "2023-09-27" @default.
• W2950441723 title "Theory of The Double Layer in Water-in-Salt Electrolytes" @default.
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