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- W2950458275 abstract "In this work, it is presented a review on several mechanistic aspects of the electrochemistry of quinones. It is discussed how the reduced intermediates, the radical anion and dianion, can be stabilized by non-covalent interactions. The intrinsic stability is a factor which can be controlled by selecting appropriately structures containing electron-withdrawing substituents, or β-hydroxy groups in possibility to establish intramolecular hydrogen bonds with the negative oxygen of the quinone reduced intermediates. Alternatively, a higher degree of stabilization can be gained when external hydrogen bonding donors are present in the medium of reaction. Weak and strong hydrogen bonding interactions are possible, however, overshooting the limit of strong interactions, proton transfer processes can occurs following a wide variety of mechanisms, whose pathway depends on the relationship between basicity of the reduced species and acidity of the proton donors." @default.
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- W2950458275 date "2007-08-02" @default.
- W2950458275 modified "2023-10-07" @default.
- W2950458275 title "Modifying the Reactivity of Reduced Intermediates of Quinones by Structural Changes and Intra and Inter Molecular Hydrogen Bonding" @default.
- W2950458275 doi "https://doi.org/10.1149/1.2753288" @default.
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