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- W2950465093 abstract "Despite a well-developed and growing body of work in copper catalysis, the potential of copper to serve as a photocatalyst remains underexplored. Here we describe a photoinduced copper-catalyzed method for coupling readily available racemic tertiary alkyl chloride electrophiles with amines to generate fully substituted stereocenters with high enantioselectivity. The reaction proceeds at –40°C under excitation by a blue light-emitting diode and benefits from the use of a single, Earth-abundant transition metal acting as both the photocatalyst and the source of asymmetric induction. An enantioconvergent mechanism transforms the racemic starting material into a single product enantiomer." @default.
- W2950465093 created "2019-06-27" @default.
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- W2950465093 date "2016-06-01" @default.
- W2950465093 modified "2023-09-27" @default.
- W2950465093 title "ChemInform Abstract: Asymmetric Copper-Catalyzed C-N Cross-Couplings Induced by Visible Light." @default.
- W2950465093 cites W2278002274 @default.
- W2950465093 doi "https://doi.org/10.1002/chin.201629148" @default.
- W2950465093 hasPublicationYear "2016" @default.
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