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- W2950502097 abstract "A series of porous carbon nanosheets having abundant micropore, nanoscale thickness and doped nitrogen were synthesized using asphaltene by three different facile routes. The three carbon nanosheets exhibited high CO2 adsorption capacity of 4.0, 4.3, 3.6 mmol/g (25 °C, 1 bar) and 5.3, 6.3, 5.1 mmol/g (0 °C, 1 bar), which should be ascribed to their developed microporous structures and surface nitrogen-containing groups. In order to evaluate their practical application, the separation performance of CO2 from CO2/N2 and CO2/CH4 was investigated according to breakthrough curves under simulate post-combustion flue gas and coalbed methane, it showed CO2 adsorption quantities at 25 °C from CO2/N2 (15/85, v/v) and CO2/CH4 (10/90, v/v) reached up to 1.22 mmol/g and 1.18 mmol/g. Furthermore, the selectivity factors for CO2 compared with N2 and CH4 were demonstrated as 15.3 and 7.3 by both ideal adsorbed solution theory model and initial slope method. Moreover, these porous carbon nanosheets could be easily regenerated and showed good stability in >10 times adsorption-desorption cycle, suggesting it promising adsorbents for CO2 capture." @default.
- W2950502097 created "2019-06-27" @default.
- W2950502097 creator A5003486476 @default.
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- W2950502097 date "2019-10-01" @default.
- W2950502097 modified "2023-10-10" @default.
- W2950502097 title "Nitrogen-doped asphaltene-based porous carbon nanosheet for carbon dioxide capture" @default.
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- W2950502097 doi "https://doi.org/10.1016/j.apsusc.2019.06.194" @default.
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