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- W295055319 abstract "The methanation of CO2 as a relevant strategy for energy storage has been studied by operando X-ray absorption spectroscopy under dynamic H2/CO2 and CO2 reaction atmospheres. A typical CO2 conversion of 81% was reached at 400 °C with a 23 wt.-% Ni/CaO–Al2O3 catalyst, yielding 80% of CH4. The operando XAS experiment under working conditions revealed pronounced structural changes, e.g., a fast bulk oxidation of the Ni particles after removal of H2 from the H2/CO2 (4:1) gas stream. A lower performance of the catalyst was observed in the subsequent methanation cycle due to the presence of a residual oxidized fraction of Ni." @default.
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- W295055319 date "2015-07-01" @default.
- W295055319 modified "2023-10-13" @default.
- W295055319 title "Methanation of CO2: Structural response of a Ni-based catalyst under fluctuating reaction conditions unraveled by operando spectroscopy" @default.
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- W295055319 doi "https://doi.org/10.1016/j.jcat.2015.04.006" @default.
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