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• W2950656985 endingPage "1997" @default.
• W2950656985 startingPage "1995" @default.
• W2950656985 abstract "The asymmetric total synthesis of the originally proposed structure of gymnangiamide, a cytotoxic pentapeptide isolated from the marine hydroid Gymnangium regae Jaderholm, has been achieved. Key to the synthesis was the use of asymmetric hydrogenation of α-substituted β-ketoesters through dynamic kinetic resolution for the preparation of nonproteinogenic chiral amino acids. The disparity of the NMR spectra between the synthetic material containing the l-serine residue and the natural product required a revision of the proposed structure." @default.
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• W2950656985 date "2009-04-08" @default.
• W2950656985 modified "2023-09-23" @default.
• W2950656985 title "Asymmetric Total Synthesis and Stereochemical Revision of Gymnangiamide" @default.
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• W2950656985 doi "https://doi.org/10.1021/ol900184d" @default.
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