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• W2950659950 abstract "Expanded porphyrin analogues with unique figure-eight conformation were prepared by way of useful pyrrole intermediates such as bis(azafulvene)s and 2-borylpyrrole. Supramolecular chirogenesis of cyclooctapyrrole O1 with 32π-cycloconjugation was successfully applied to determine absolute configuration of chiral carboxylic acids. Dinuclear CuII complex of cyclooctapyrrole O2 with interrupted π-conjugation was resolved by HPLC into enantiomers and their helical handedness was determined by theoretical simulation of their CD spectral pattern. Enantioselective induction of helicity in the metal helicate formation in the presence of a chiral promoter was demonstrated by using (R)-(+)-1-(1-phenyl)ethylamine that favoured P, P helicity. Dinuclear CoII complexes of cyclotetrapyrroletetrapyridine O3 were found to be substitution labile and pick up amino acid anions in water. Those amino acid complexes of O3Co 2 were rendered to adopt a particular unidirectional helical conformation preferentially depending on the ligated amino acid anion." @default.
• W2950659950 created "2019-06-27" @default.
• W2950659950 creator A5004001379 @default.
• W2950659950 date "2013-11-04" @default.
• W2950659950 modified "2023-09-24" @default.
• W2950659950 title "ChemInform Abstract: Helical Chirality Induction of Expanded Porphyrin Analogues" @default.
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• W2950659950 doi "https://doi.org/10.1002/chin.201347222" @default.
• W2950659950 hasPublicationYear "2013" @default.
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