Matches in SemOpenAlex for { <https://semopenalex.org/work/W2950706773> ?p ?o ?g. }
- W2950706773 abstract "Adsorption sites of molecules critically determine the electric/photonic properties and its stability of heterogeneous molecule-metal interfaces. Then, selectivity of adsorption site is essential for development of the fields including organic electronics, catalysis, and biology. However, due to current technical limitations, site-selectivity remains a major challenge because of difficulty in precise selection of meaningful one among the sites. Here, we report the single site-selection at a single-molecule junction by performing newly developed hybrid technique: simultaneous characterization of surface enhanced Raman scattering (SERS) and current-voltage (I-V) measurements. The I-V response of 1,4-benzenedithiol junctions, reveals the existence of three meta-stable states arising from different adsorption sites. Notably, correlated SERS measurements show selectivity towards one of the adsorption sites, bridge sites. This site-selectivity represents an essential step towards the reliable integration of individual molecules on metallic surfaces. Furthermore, the hybrid spectro-electric technique reveals the dependence of the SERS intensity on the strength of the molecule-metal interaction, showing the interdependence between the optical and electronic properties in single-molecule junctions." @default.
- W2950706773 created "2019-06-27" @default.
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- W2950706773 date "2016-01-13" @default.
- W2950706773 modified "2023-09-23" @default.
- W2950706773 title "Site selection in single-molecule junction for highly reproducible molecular electronics" @default.
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- W2950706773 doi "https://doi.org/10.48550/arxiv.1601.03460" @default.
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