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- W2950874591 abstract "Enantiodivergent catalyst systems were developed using metals with different ionic radii and a multifunctional brucine diol (BD) ligand. The catalytic use of purported 1:1 Cu-BD complexes in the 1,3-dipolar cycloaddition of azomethine ylides with chalcones resulted in the selective formation of endo-pyrrolidines in 87–96% ees with an absolute stereochemical outcome of (2R,3S,4R,5S). In contrast, an opposite absolute stereochemical outcome was observed by using the catalysts derived from Ag(I) salts and BD. The demonstration of enantiodivergent approaches to a broad class of substrates/reaction types underlines their synthetic value in asymmetric synthesis." @default.
- W2950874591 created "2019-06-27" @default.
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- W2950874591 date "2016-07-01" @default.
- W2950874591 modified "2023-09-27" @default.
- W2950874591 title "ChemInform Abstract: Enantiodivergent Brucine Diol-Catalyzed 1,3-Dipolar Cycloaddition of Azomethine Ylides with α,β-Unsaturated Ketones." @default.
- W2950874591 cites W2280498771 @default.
- W2950874591 doi "https://doi.org/10.1002/chin.201631145" @default.
- W2950874591 hasPublicationYear "2016" @default.
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