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- W2950882205 abstract "Synchrotron X-ray, neutron powder diffraction, and magnetic susceptibility measurements have been used to characterize the Ln2LiRuO6 (Ln = Pr, Nd, Sm, Eu, Gd, and Tb) double perovskites. All compositions have the monoclinic P21/n superstructure with a fully ordered arrangement of Li+ and Ru5+ cations. As the Ln-size decreases, the lattice volume decreases due to the increased tilting of the octahedra, but the Li−O and Ru−O distances remain constant. Antiferromagnetic transitions with Néel temperatures in the 20−35 K range were observed for all compositions, except for Gd2LiRuO6, which does not order down to 5 K. Nd2LiRuO6 shows a field-induced ferrimagnetic transition at ∼4 Tesla. The Ln = Pr, Nd, and Tb materials have type I magnetic structures with coupled spin ordering on the Ln and Ru sublattices. Critical fits reveal that the Ln3+ sublattice magnetization shows mean field behaviour (β ≈ 0.5), whereas the Ru5+ spin order is consistent with the three-dimensional Heisenberg model (β = 0.31−0.35)." @default.
- W2950882205 created "2019-06-27" @default.
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- W2950882205 date "2008-12-23" @default.
- W2950882205 modified "2023-10-17" @default.
- W2950882205 title "Coupled Spin Ordering in the Ln<sub>2</sub>LiRuO<sub>6</sub> Double Perovskites" @default.
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- W2950882205 doi "https://doi.org/10.1021/cm8020935" @default.
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