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- W2951043964 abstract "Abstract The specific ionic conductivity, σ, of the solid electrolyte RbAg 4 I 5 was determined by four-probe impedance measurements in the temperature range 28 ⩽ T ⩽ 299 K. Good agreement was obtained with previous two-probe σ data at temperatures above the β-γ phase transition temperature T β-γ = 121.75 K. Between T β-γ and about T = 109±1 K, a decrease of σ by 2–3 orders of magnitude occurred. At T ⩽ 109 K, a distinct change in the activation energy of σ was observed with almost temperature-independent mobility of the conducting Ag + ions in this low temperature range. This behaviour is explained by a possible glass-like transition occurring at T g ≈ 109 K, and a barrierless tunnelling mechanism via TLS states (two-level tunnelling system) below T g . The implications of the low-temperature conductivity of solid electrolytes for electrochemical studies in this temperature range are discussed." @default.
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- W2951043964 date "1990-09-25" @default.
- W2951043964 modified "2023-09-25" @default.
- W2951043964 title "ChemInform Abstract: Low-Temperature Ion Conductivity of RbAg4I5." @default.
- W2951043964 cites W2058337515 @default.
- W2951043964 doi "https://doi.org/10.1002/chin.199039009" @default.
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