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• W2951241569 endingPage "19858" @default.
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• W2951241569 abstract "The photodissociation dynamics of four chlorine-containing compounds was studied by the ion imaging technique. Two compounds, ClNO and (CH3)3COCl, exhibited strong anisotropy, and the kinetic energy distributions for Cl(2P3/2) and Cl*(2P1/2) were indistinguishable. For CCl4 and SOCl2 the kinetic energy distributions of Cl and Cl* were very different. In all cases most of the chlorine atoms were released in their ground 2P3/2 state. A general explanation is given based on these data and those of others. The process is described in terms of three states whose energies are in the following order: the ground state, a state correlating with Cl*, and a state correlating with Cl. Sooner or later the Cl state must cross the Cl* state. If the crossing is sooner, i.e. in the Franck−Condon region, Cl and Cl* will have different translational energy distributions. If the crossing is later, i.e. at long distances, Cl and Cl* will have descended a repulsive surface and reached their asymptotic and nearly equal kinetic energies." @default.
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• W2951241569 date "1996-01-01" @default.
• W2951241569 modified "2023-10-10" @default.
• W2951241569 title "Ion Imaging of the Photodissociation of Chlorine-Containing Molecules" @default.
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• W2951241569 doi "https://doi.org/10.1021/jp9609343" @default.
• W2951241569 hasPublicationYear "1996" @default.
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