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• W2951282283 abstract "The binding of metal ions to heteroatomic centers of biomolecules has been utilized as a probe of metal ion effects in living systems. This article focuses on the effect of N-coordination by transition metals, especially Pt(II), Co(III), Cr(III), on isotopic C(2)−H or C(8)−H exchange of imidazoles, thiazoles, and purines. The usual reactivity trend, protonated ≫ metalated ≫ neutral substrate, is excepted for Cr(III)/1-methylimidazole, where Cr(III) activates stronger than H+. An interplay of factors is considered, including metal-to-ligand back-bonding, electronic structure of metal ions, and differences in crystal field stabilization energy." @default.
• W2951282283 created "2019-06-27" @default.
• W2951282283 creator A5007594566 @default.
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• W2951282283 date "2000-07-06" @default.
• W2951282283 modified "2023-10-10" @default.
• W2951282283 title "Metal Ion Effects in Isotopic Hydrogen Exchange in Biologically Important Heterocycles" @default.
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• W2951282283 doi "https://doi.org/10.1021/ar970209q" @default.
• W2951282283 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/11041831" @default.
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