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- W2951310636 abstract "Chiral phosphoric acid diesters arguably constitute the most exploited class of catalysts in asymmetric Bronsted acid catalysis. Despite being highly investigated for their acidic properties, these compounds display an amphoteric nature, which has instead been considerably overlooked. The potential of this dichotomous polarity has recently been disclosed and applied to the development of novel reaction modes in organocatalysis. In this account, we present our recent advances in this area, focusing on the establishment of heterodimeric interactions toward the nucleophilic activation of carboxylic acids, thiocarboxylic acids and ketones (via their enols) in asymmetric transformations. 1Introduction 2Discovery of Heterodimeric Self-Assemblies 3Activation of Carboxylic Acids 3.1The Enantioselective Carboxylysis of Aziridines 3.2An Asymmetric Hydrolysis of Epoxides 4Activation of Thiocarboxylic Acids 5Enol Catalysis 5.1Asymmetric Michael Addition 5.2Asymmetric α-Amination 5.3Asymmetric α-Allylation 6Concluding Remarks" @default.
- W2951310636 created "2019-06-27" @default.
- W2951310636 creator A5034457900 @default.
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- W2951310636 date "2016-06-01" @default.
- W2951310636 modified "2023-10-01" @default.
- W2951310636 title "ChemInform Abstract: Phosphoric Acid Based Heterodimers in Asymmetric Catalysis" @default.
- W2951310636 cites W2320361128 @default.
- W2951310636 doi "https://doi.org/10.1002/chin.201625256" @default.
- W2951310636 hasPublicationYear "2016" @default.
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