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• W2951468032 startingPage "025001" @default.
• W2951468032 abstract "We theoretically study the electrolyte Seebeck effect in the vicinity of a heated metal nanostructure, such as the cap of an active Janus colloid in an electrolyte, or gold- coated interfaces in optofluidic devices. The thermocharge accumulated at the surface varies with the local temperature, thus modulating the diffuse part of the electric double layer. On a conducting surface with non-uniform temperature, the isopotential condition imposes a significant polarization charge within the metal. Surprisingly, this does not affect the slip velocity, which takes the same value on insulating and conducting surfaces. Our results for specific-ion effects agree qualitatively with recent observations for Janus colloids in different electrolyte solutions. Comparing the thermal, hydrodynamic, and ion diffusion time scales, we expect a rich transient behavior at the onset of thermally powered swimming, extending to microseconds after switching on the heating." @default.
• W2951468032 created "2019-06-27" @default.
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• W2951468032 date "2018-02-02" @default.
• W2951468032 modified "2023-10-18" @default.
• W2951468032 title "Nanoscale Seebeck effect at hot metal nanostructures" @default.
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• W2951468032 doi "https://doi.org/10.1088/1367-2630/aaa266" @default.
• W2951468032 hasPublicationYear "2018" @default.
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