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- W2951599286 abstract "An efficient strategy for the in situ generation of heterocyclic ortho-quinodimethanes (oQDMs) from 2-methyl-heteroarene-3-carboxylic esters by N-heterocyclic carbene (NHC) catalysis is disclosed. These heterocyclic oQDMs undergo highly enantioselective [4 + 2] annulation reactions with isatin-derived ketimines to afford optically pure heteroarene-fused δ-lactams bearing a quaternary stereogenic center. The main features of this reaction include challenging direct C(sp3)–H bond functionalizations, excellent enantioselectivities, readily available starting materials, mild reaction conditions, high efficiency, and operational simplicity." @default.
- W2951599286 created "2019-06-27" @default.
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- W2951599286 date "2016-12-01" @default.
- W2951599286 modified "2023-09-27" @default.
- W2951599286 title "ChemInform Abstract: N-Heterocyclic Carbene Catalyzed [4 + 2] Annulation Reactions with in situ Generated Heterocyclic ortho-Quinodimethanes." @default.
- W2951599286 cites W2460521252 @default.
- W2951599286 doi "https://doi.org/10.1002/chin.201652187" @default.
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