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• W2951660272 abstract "The asymmetric allylboration of N-H aldimines with optically pure trans-4-substituted-2-boryl-1,3-dienes 6 is described. These organoboranes 6 serve as near-perfect asymmetric allylborating agents for N-H aldimines for the preparation of anti-1,2-disubstituted-3,4-pentadien-1-amines 11 as essentially single diastereomers in enantiomerically pure form (>98% de, ≥98% ee). Enantiomerically pure cis-2,3-disubstitued piperidines 12 and α,β-disubstituted-β-amino acids 17 are readily prepared through the standard protocols. A novel Ru-catalyzed hydroamination provides trans-4,5-disubstituted-1-pyrrolines 21 from 11." @default.
• W2951660272 created "2019-06-27" @default.
• W2951660272 creator A5001989466 @default.
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• W2951660272 date "2014-07-08" @default.
• W2951660272 modified "2023-10-07" @default.
• W2951660272 title "(<i>E</i>)-2-Boryl 1,3-Dienes from the 10-TMS-9-BBDs: Highly Selective Reagents for the Asymmetric Synthesis of <i>anti</i>-α,β-Disubstituted β-Allenylamines from the Allylboration of Aldimines" @default.
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• W2951660272 doi "https://doi.org/10.1021/ol501892a" @default.
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