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- W2951805671 abstract "The vibrational, rotational, and translational energy distributions for the CO photofragments from the 193, 248, and 308 nm photolysis of Ni(CO)4 in a supersonic molecular beam have been determined by vacuum ultraviolet laser‐induced fluorescence. The measured product energy distributions appeared to be statistical, with equilibrium between the degrees of freedom investigated. The distributions were significantly colder than those calculated with a microcanonical statistical model using published bond energies. To model the measured distributions, it was necessary to postulate that the unsaturated nickel carbonyl products are formed in a stable electronically excited state. By using an excited state energy consistent with published fluorescence experiments, excellent agreement was obtained between the measured distributions and those calculated using a microcanonical statistical model. These results indicate that for 193 nm photolysis, essentially all of the Ni(CO)n products are electronically excited, wi..." @default.
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- W2951805671 date "2010-09-01" @default.
- W2951805671 modified "2023-09-23" @default.
- W2951805671 title "ChemInform Abstract: State Resolved Photofragmentation of Ni(CO)4 at 193, 248, and 308 nm: A Detailed Study of the Photodissociation Dynamics." @default.
- W2951805671 cites W1993598553 @default.
- W2951805671 doi "https://doi.org/10.1002/chin.199113235" @default.
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