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- W2951878518 abstract "Abstract The ambident nature of the electrophile generated in a reaction system controls the outcome of a reaction. Electrophilic nitrenium ion which is convertible to carbenium ion via resonance was in situ generated by the reactions of iodine(III)‐reagent PhI(OAc) 2 and arylsulfonamides. The nucleophile added in the reaction controls the reaction for the regiospecific ortho C−H arylation or C 2 ‐H arylation. The electron rich arenes react with carbenium ion (electrophiles) to undergo C−H arylation. Electron donating effect (+I or +R effect) of the substituents on sulfonamide stabilizes the carbenium ion to favor oxidative coupling reaction with nucleophiles. Overall, the feasibility of C 2 ‐H arylation of the sulfonamides has been demonstrated by steric and electronic factor that facilitates C−H arylation of sulfonamides." @default.
- W2951878518 created "2019-06-27" @default.
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- W2951878518 date "2019-06-19" @default.
- W2951878518 modified "2023-09-27" @default.
- W2951878518 title "Steric and Electronic Effect on C 2 ‐H Arylation of Sulfonamides" @default.
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- W2951878518 doi "https://doi.org/10.1002/slct.201900944" @default.
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