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• W2952307406 abstract "Laser-ablated Ge atoms and H2 molecules in excess neon and argon react during condensation to produce GeH1,2,3,4 as identified from infrared spectra with D2 and HD substitution, and from agreement with frequencies determined in recent gas-phase GeH and GeH2 fluorescence spectra and DFT calculations. The novel digermanium species Ge2H2 and Ge2H4 are formed in further reactions. Identification of Ge2H2 with the dibridged structure and Ge2H4 in the trans-bent C2h form is made possible by isotopic substitution and quantum chemical frequency calculations, which demonstrate the value of a close working relationship between experiment and theory. The photosensitive GeH3- anion is formed through electron capture by a GeH3 radical. All four germanium deuterides are observed in pure deuterium, which shows that further GeD and GeD2 reactions with D2 may require activation energy." @default.
• W2952307406 created "2019-06-27" @default.
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• W2952307406 date "2002-05-24" @default.
• W2952307406 modified "2023-09-27" @default.
• W2952307406 title "Infrared Spectra of the Novel Ge₂H₂ and Ge₂H₄ Species and the Reactive GeH_1,2,3 Intermediates in Solid Neon, Deuterium and Argon" @default.
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• W2952307406 doi "https://doi.org/10.1021/jp020219v" @default.
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