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- W2952583149 abstract "Concise total syntheses of naturally occurring nothapodytine B (1, mappicine ketone) and (−)-mappicine (3) are detailed. The approach is based on the implementation of a room-temperature, inverse electron demand Diels−Alder reaction of the N-sulfonyl-1-aza-1,3-butadiene 11 for assemblage of a pyridone D ring precursor central to the structure. A Friedlander condensation is utilized for constructing the AB ring system of 1 and 3. An acid-catalyzed reaction sequence is used to accomplish a deprotection with subsequent ring-closure for introduction of the C ring in a single step." @default.
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- W2952583149 date "1998-01-30" @default.
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- W2952583149 title "Total Synthesis of Nothapodytine B and (−)-Mappicine" @default.
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- W2952583149 doi "https://doi.org/10.1021/ja973007y" @default.
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