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- W2952599617 abstract "The CIDEP spectrum of acetone has been studied by means of time‐resolved EPR over a wide range of temperature. It was found that the spectrum varied remarkably depending on temperature indicating that different CIDEP mechanisms are involved at different temperatures. The CIDEP mechanisms operating in each temperature region are determined quantitatively mainly from the simulations of the spectra and their dependence on the diffusion constant of the solvent; from room temperature to −90 °C, the radical pair mechanism involving S–T0 mixing (ST0M)is always dominant, but the triplet mechanism and the radical pair mechanism involving S–T−1 mixing (ST−1M)become important above and below −45 °C, respectively. The relative importance of ST−1M as compared with ST0M determined below −60 °C is in good agreement with the prediction of the theory. We have also found two interesting phenomena that relatively strong E/A peaks appeared in the center portion of the complete E/A spectrum around −45 °C, and that the line sh..." @default.
- W2952599617 created "2019-06-27" @default.
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- W2952599617 date "1988-05-24" @default.
- W2952599617 modified "2023-09-25" @default.
- W2952599617 title "ChemInform Abstract: Temperature Dependence of the CIDEP Spectrum of Acetone" @default.
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- W2952599617 doi "https://doi.org/10.1002/chin.198821093" @default.
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