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- W2952998103 abstract "A protocol involving a gold(I)-catalyzed reaction to elaborate cyclic frames by selective trimerization reactions of N-allenylsulfonamides is reported. Efficiency in the formation of the target [2+2+2] products depends on the concentration of the reagents, the nature of the ancillary ligand on the gold catalyst, and, to a significant extent, on the selection of a low reaction temperature. This singular catalytic allene cycloaddition gives adducts in high isolated yields. In addition to representing a new gold-catalyzed reaction, the reported allenamide cyclotrimerization offers a significant extension to the scant number of allenes that have effectively entered this cyclization mode by use of other metal-catalyzed reactions. Upon aromatization of the assembled adducts, the overall reaction matches the outcome of related and widely investigated alkyne trimerization reactions." @default.
- W2952998103 created "2019-06-27" @default.
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- W2952998103 date "2016-05-01" @default.
- W2952998103 modified "2023-09-27" @default.
- W2952998103 title "ChemInform Abstract: Gold-Catalyzed Allenamide [2 + 2 + 2]-Cyclotrimerization." @default.
- W2952998103 cites W2183157555 @default.
- W2952998103 doi "https://doi.org/10.1002/chin.201622033" @default.
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