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- W2953014922 abstract "Catalytic enantioselective Kinugasa reactions between acyclic and, for the first time, cyclic nitrones and terminal alkynes are described herein. A catalytic amount of the readily available PINAP/CuX complexes, generated in situ, efficiently catalyzed the Kinugasa reactions, leading to a series of β-lactams with good enantioselectivities and moderate diastereoselectivities and yields. A broad range of nitrones and terminal alkynes, including the seldom reported alkyl-substituted alkynes, were tolerated under the reaction conditions. Further investigations proved that the PINAP/CuX catalytic system enabled the synthesis of monobactams on the gram scale (without loss of stereoselectivity and yield) and also both enantiomers by the appropriate choice of readily available atropisomeric N-PINAP ligands." @default.
- W2953014922 created "2019-06-27" @default.
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- W2953014922 date "2016-08-01" @default.
- W2953014922 modified "2023-10-04" @default.
- W2953014922 title "ChemInform Abstract: Studies on the Enantioselective Kinugasa Reaction: Efficient Synthesis of β-Lactams Catalyzed by N-PINAP/CuX Complexes." @default.
- W2953014922 cites W2319801641 @default.
- W2953014922 doi "https://doi.org/10.1002/chin.201636098" @default.
- W2953014922 hasPublicationYear "2016" @default.
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