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• W2953037620 abstract "The solution structures of the radical anion and the radical cation of the donor-acceptor molecules 3,4-di(1,3-dithiol-2-ylidene)-4-phenylbut-1-ene-1,1-dicarbonitrile (1) and 3,4-di(1,3-dithiol-2-ylidene)-4-phenylbut-1-ene-1,1,2-tricarbonitrile (2) are discussed based on cyclovoltammetric and ESR/ENDOR measurements. It is shown that the spin population of the radical anions is limited to the di- and tricyanoethene moiety and the coplanar 1,3-dithiole at C(3), whereas that of the radical cations resides mainly inside the two 1,3-dithiole rings. The energies of the long-wave bands in the electronic-absorption spectra of 1 and 2 correspond to the differences between the oxidation and reduction potentials and thus point to a charge-transfer character of these transitions." @default.
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• W2953037620 date "1994-08-10" @default.
• W2953037620 modified "2023-09-27" @default.
• W2953037620 title "Solution Structure of One-Electron Reduced and Oxidized Molecules with Twisted Donor and Acceptor Moieties" @default.
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• W2953037620 doi "https://doi.org/10.1002/hlca.19940770524" @default.
• W2953037620 hasPublicationYear "1994" @default.
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